In 1999, the couple founded Exploring the Arts, a non-profit organization that supports arts education through more than 50 school partnerships in New York and Los Angeles.

"I happen to be one of those lucky people who can honestly say that dreams do come true. Being able to work with my husband, Tony Bennett, has been one such dream," Crow wrote in a 2013 op-ed for The Huffington Post. "Together we founded a nonprofit organization, Exploring the Arts (ETA), to transform the lives of young people through arts education."

Bennett and Crow also opened the Frank Sinatra School of the Arts in 2001—named after one of Bennett's close friends—in his hometown of Queens, N.Y., where Crow served as a social studies teacher and assistant principal.